文章编号:1009−444X(2023)02−0113−07光−臭氧催化氧化型SiC泡沫陶瓷的制备及其在左氧氟沙星降解中的应用邹敬桃,李旋坤,杨洁,魏铭飞,张文启,李光辉(上海工程技术大学化学化工学院,上海201620)摘要:针对抗生素难以降解而造成环境污染问题,以左氧氟沙星(Levofloxacin,LEV)为目标污染物,制备Ce-TiO2/SiC泡沫陶瓷复合材料,并由此构建光催化臭氧氧化耦合体系(Ce-TiO2/SiC+LED+O3).结果表明,该耦合体系能有效降解LEV,去除率为99%,化学需氧量(ChemicalOxygenDemand,COD)降解率高达85.9%.该耦合体系体现了较高的协同效应,其一级反应动力学速率常数大于臭氧氧化(O3)与光催化(Ce-TiO2/SiC+LED)之和.另外,Ce-TiO2/SiC泡沫陶瓷的稳定性实验表明,在5次重复使用实验后,光催化臭氧氧化活性基本不变.关键词:光催化臭氧氧化;COD降解;左氧氟沙星中图分类号:O643.36文献标志码:APreparationofphotocatalyticozonationSiCfoamanditsapplicationinlevofloxacindegradationZOUJingtao,LIXuankun,YANGJie,WEIMingfei,ZHANGWenqi,LIGuanghui(SchoolofChemistryandChemicalEngineering,ShanghaiUniversityofEngineeringScience,Shanghai201620,China)Abstract:Tosolvetheproblemofenvironmentalpollutioncausedbythedifficultdegradationofantibiotics,Ce-TiO2/SiCfoamwasprepared,levofloxacin(Levofloxacin,LEV)waschosenasthetargetpollutant,andaphotocatalyticozonationcouplingsystem(Ce-TiO2/SiC+LED+O3)wasstudied.TheresultsshowthatthecouplingsystemcaneffectivelydegradeLEV,theLEVremovalwas99%andthechemicaloxygendemand(COD)removalwasashighas85.9%.Thecouplingsystemshowedagoodsynergisticeffect,anditsfirst-orderreactionkineticrateconstantwasgreaterthanthesumofozonation(O3)andphotocatalysis(Ce-TiO2/SiC+LED).Inaddition,thestabilityexperimentofCe-TiO2/SiCfoamshowedthatthephotocatalyticozonationactivityisbasicallyunchangedafterfivereuses.Keywords:photocatalyticozonation;chemicaloxygendemand(COD)removal;levofloxacin(LEV)左氧氟沙星(Levofloxacin,LEV)是一种氟喹诺酮类(Fluoroquinolones,FQs)抗生素,用于治疗被细菌感染的人和动物[1].近年来,有研究者发现各类水体中FQs浓度(质量分数,全文同)逐渐增加[2].环境中残留的抗生素导致耐药性基因和耐药性细菌的产生和...