第44卷第2期2023年2月Vol.44No.2Feb.,2023发光学报CHINESEJOURNALOFLUMINESCENCE基于上转换发光的Y7O6F9∶Er,Yb/PAN复合纤维温度传感特性赵昕,刘哲,林海,李德胜*(大连工业大学信息科学与工程学院,辽宁大连116034)摘要:通过水热法配合高温煅烧合成了斜方晶系Y7O6F9∶Er,Yb晶体,该晶体可实现高效上转换发光且具有良好的高分子亲和性。利用高压静电纺丝技术将Y7O6F9∶Er,Yb晶体颗粒与高分子化合物聚丙烯腈(PAN)复合,制备出了兼备温度传感特性、柔韧性和灵活性的Y7O6F9∶Er,Yb/PAN纤维。977nm激光激发下,晶体颗粒和复合纤维在303~433K温度范围内均展示出高效的上转换发光和良好的温度传感特性,且复合纤维在测温范围内表现出优于晶体颗粒的温度灵敏度和分辨率。在303K温度下有最大绝对灵敏度值1.143%·K‒1,在433K温度下有最小的分辨率0.15K。因此,具有柔韧性的复合纤维既有良好温度传感特性又可任意调节形态,适应复杂多样的应用环境,是可应用于实现智能穿戴领域温度传感性能的有效候选材料。关键词:Y7O6F9∶Er,Yb/PAN复合纤维;高压静电纺丝;上转换发光;温度传感中图分类号:O482.31文献标识码:ADOI:10.37188/CJL.20220350TemperatureSensingCharacteristicsofY7O6F9∶Er,Yb/PANCompositeFibersBasedonUp-conversionLuminescenceZHAOXin,LIUZhe,LINHai,LIDesheng*(SchoolofInformationScienceandEngineering,DalianPolytechnicUniversity,Dalian116034,China)*CorrespondingAuthor,E-mail:deshengli80@163.comAbstract:Y7O6F9∶Er,Yborthorhombiccrystalsweresynthesizedbyhydrothermalmethodandhigh-temperaturecalcination,whichachievesefficientup-conversionluminescenceandhassatisfactorypolymeraffinity.Y7O6F9∶Er,Yb/PANcompositefiberswithhightemperaturesensingproperties,andcommendableflexibilitywerepreparedbyhighvoltageelectrospinningtechnology.Undertheexcitationof977nmlaser,thecompositefibersshowefficientup-conversionluminescenceandbettertemperaturesensingperformancethancrystalsinthetemperaturerangeof303Kto433K.Withinthetemperaturerangeofmeasurement,themaximumvalueofSAandSRofY7O6F9∶Er,Ybcrystalsis0.720%·K‒1and1.142%·K‒1,andtheminimumtemperatureresolutionwas0.37K.ThemaximumvalueofSAandSRofY7O6F9∶Er,Yb/PANcompositefibersis0.811%·K‒1an...